Sims 3 on Mac: Application startup failed
Instead of launch of one the last EP, you should use the basic game. Navigate to ”Applications” > then to the folder ”The Sims 3” and find the icon for the main game. Launch from there or drag a copy into the dock. It should work then ..

If this does not help, something is wrong with your permission and file.
How to fix your permissions, read more

You can try this too!
Go where the file is located. / Applications / The Sims 3.localized / The Sims 3 Master Suite
copy the update_gamekeys.reg

Put it on the desktop, take the file from the desktop and put it into the following folder.
/ Users / YourName / Library / Preferences / The Sims 3 Preferences /

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